Raman scattering of InAs/AlAs quantum dot superlattices grown on (001) and (311)B GaAs surfaces

Abstract

We present a comparative analysis of Raman scattering by acoustic and optical phonons in InAs/AlAs quantum dot superlattices grown on (001) and (311)B GaAs surfaces. Doublets of folded longitudinal acoustic phonons up to the fifth order were observed in the Raman spectra of (001)- and (311)B-oriented quantum dot superlattices measured in the polarized scattering geometries. The energy positions of the folded acoustic phonons are well described by the elastic continuum model. Besides the acoustic phonons, the spectra display features related to confined transverse and longitudinal optical as well as interface phonons in quantum dots and spacer layers. Their frequency positions are discussed in terms of phonon confinement, elastic stress, and atomic intermixing.

Original language	English
Article number	476
Journal	Nanoscale Research Letters
Volume	7
DOIs	https://doi.org/10.1186/1556-276X-7-476
Publication status	Published - 17 Sep 2012
Externally published	Yes

Keywords

Nanocrystals
Nanoparticles
Phonons
Quantum dots
Raman scattering spectroscopy

ASJC Scopus subject areas

Materials Science(all)
Condensed Matter Physics

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10.1186/1556-276X-7-476

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@article{3975817e8049433b893cc8c993874125,

title = "Raman scattering of InAs/AlAs quantum dot superlattices grown on (001) and (311)B GaAs surfaces",

abstract = "We present a comparative analysis of Raman scattering by acoustic and optical phonons in InAs/AlAs quantum dot superlattices grown on (001) and (311)B GaAs surfaces. Doublets of folded longitudinal acoustic phonons up to the fifth order were observed in the Raman spectra of (001)- and (311)B-oriented quantum dot superlattices measured in the polarized scattering geometries. The energy positions of the folded acoustic phonons are well described by the elastic continuum model. Besides the acoustic phonons, the spectra display features related to confined transverse and longitudinal optical as well as interface phonons in quantum dots and spacer layers. Their frequency positions are discussed in terms of phonon confinement, elastic stress, and atomic intermixing.",

keywords = "Nanocrystals, Nanoparticles, Phonons, Quantum dots, Raman scattering spectroscopy",

author = "Alexander Milekhin and Nikolay Yeryukov and Alexander Toropov and Dmitry Dmitriev and Evgeniya Sheremet and Zahn, {Dietrich R.T.}",

year = "2012",

month = sep,

day = "17",

doi = "10.1186/1556-276X-7-476",

language = "English",

volume = "7",

journal = "Nanoscale Research Letters",

issn = "1931-7573",

publisher = "Springer New York",

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TY - JOUR

T1 - Raman scattering of InAs/AlAs quantum dot superlattices grown on (001) and (311)B GaAs surfaces

AU - Milekhin, Alexander

AU - Yeryukov, Nikolay

AU - Toropov, Alexander

AU - Dmitriev, Dmitry

AU - Sheremet, Evgeniya

AU - Zahn, Dietrich R.T.

PY - 2012/9/17

Y1 - 2012/9/17

N2 - We present a comparative analysis of Raman scattering by acoustic and optical phonons in InAs/AlAs quantum dot superlattices grown on (001) and (311)B GaAs surfaces. Doublets of folded longitudinal acoustic phonons up to the fifth order were observed in the Raman spectra of (001)- and (311)B-oriented quantum dot superlattices measured in the polarized scattering geometries. The energy positions of the folded acoustic phonons are well described by the elastic continuum model. Besides the acoustic phonons, the spectra display features related to confined transverse and longitudinal optical as well as interface phonons in quantum dots and spacer layers. Their frequency positions are discussed in terms of phonon confinement, elastic stress, and atomic intermixing.

AB - We present a comparative analysis of Raman scattering by acoustic and optical phonons in InAs/AlAs quantum dot superlattices grown on (001) and (311)B GaAs surfaces. Doublets of folded longitudinal acoustic phonons up to the fifth order were observed in the Raman spectra of (001)- and (311)B-oriented quantum dot superlattices measured in the polarized scattering geometries. The energy positions of the folded acoustic phonons are well described by the elastic continuum model. Besides the acoustic phonons, the spectra display features related to confined transverse and longitudinal optical as well as interface phonons in quantum dots and spacer layers. Their frequency positions are discussed in terms of phonon confinement, elastic stress, and atomic intermixing.

KW - Nanocrystals

KW - Nanoparticles

KW - Phonons

KW - Quantum dots

KW - Raman scattering spectroscopy

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JF - Nanoscale Research Letters

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