Migration of hydrogen in steel and alloys, stimulated by ionizing radiation

Abstract

A study is made of the behavior of hydrogen in stainless steel and alloys of titanium and vanadium during exposure of the metals to ionizing radiation (accelerated nitrogen ions, γ-quanta). It is shown that the radiation stimulates intensive migration of hydrogen. The cross section of the accelerated ions is 10^-16 cm². This shows that hydrogen is released from traps as a result of excitation of the electronic subsystem and vibrational degrees of freedom of the hydrogen bonds, with the excitation energy subsequently being transferred to the nuclear subsystem. A phenomenological model is proposed to describe the ionization-accelerated migration of hydrogen in metals. Gamma- and electron-stimulated dissociation of hydrogen-containing bonds inside a solid occur by the Mensell - Homer and Auger mechanisms, as well as by nonadiabatic transition and vibrational-translational exchange. The calculated probability of the migration of hydrogen by these mechanisms is found to agree well with the experimental data.

Original language	English
Pages (from-to)	1072-1078
Number of pages	7
Journal	Russian Physics Journal
Volume	37
Issue number	11
DOIs	https://doi.org/10.1007/BF00559215
Publication status	Published - Nov 1994

ASJC Scopus subject areas

Physics and Astronomy(all)

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10.1007/BF00559215

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Chernov, I. P., Mamontov, A. P., Tyurin, Y. I., & Cherdantsev, Y. P. (1994). Migration of hydrogen in steel and alloys, stimulated by ionizing radiation. Russian Physics Journal, 37(11), 1072-1078. https://doi.org/10.1007/BF00559215

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title = "Migration of hydrogen in steel and alloys, stimulated by ionizing radiation",

abstract = "A study is made of the behavior of hydrogen in stainless steel and alloys of titanium and vanadium during exposure of the metals to ionizing radiation (accelerated nitrogen ions, γ-quanta). It is shown that the radiation stimulates intensive migration of hydrogen. The cross section of the accelerated ions is 10-16 cm2. This shows that hydrogen is released from traps as a result of excitation of the electronic subsystem and vibrational degrees of freedom of the hydrogen bonds, with the excitation energy subsequently being transferred to the nuclear subsystem. A phenomenological model is proposed to describe the ionization-accelerated migration of hydrogen in metals. Gamma- and electron-stimulated dissociation of hydrogen-containing bonds inside a solid occur by the Mensell - Homer and Auger mechanisms, as well as by nonadiabatic transition and vibrational-translational exchange. The calculated probability of the migration of hydrogen by these mechanisms is found to agree well with the experimental data.",

author = "Chernov, {I. P.} and Mamontov, {A. P.} and Tyurin, {Yu I.} and Cherdantsev, {Yu P.}",

year = "1994",

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T1 - Migration of hydrogen in steel and alloys, stimulated by ionizing radiation

AU - Chernov, I. P.

AU - Mamontov, A. P.

AU - Tyurin, Yu I.

AU - Cherdantsev, Yu P.

PY - 1994/11

Y1 - 1994/11

N2 - A study is made of the behavior of hydrogen in stainless steel and alloys of titanium and vanadium during exposure of the metals to ionizing radiation (accelerated nitrogen ions, γ-quanta). It is shown that the radiation stimulates intensive migration of hydrogen. The cross section of the accelerated ions is 10-16 cm2. This shows that hydrogen is released from traps as a result of excitation of the electronic subsystem and vibrational degrees of freedom of the hydrogen bonds, with the excitation energy subsequently being transferred to the nuclear subsystem. A phenomenological model is proposed to describe the ionization-accelerated migration of hydrogen in metals. Gamma- and electron-stimulated dissociation of hydrogen-containing bonds inside a solid occur by the Mensell - Homer and Auger mechanisms, as well as by nonadiabatic transition and vibrational-translational exchange. The calculated probability of the migration of hydrogen by these mechanisms is found to agree well with the experimental data.

AB - A study is made of the behavior of hydrogen in stainless steel and alloys of titanium and vanadium during exposure of the metals to ionizing radiation (accelerated nitrogen ions, γ-quanta). It is shown that the radiation stimulates intensive migration of hydrogen. The cross section of the accelerated ions is 10-16 cm2. This shows that hydrogen is released from traps as a result of excitation of the electronic subsystem and vibrational degrees of freedom of the hydrogen bonds, with the excitation energy subsequently being transferred to the nuclear subsystem. A phenomenological model is proposed to describe the ionization-accelerated migration of hydrogen in metals. Gamma- and electron-stimulated dissociation of hydrogen-containing bonds inside a solid occur by the Mensell - Homer and Auger mechanisms, as well as by nonadiabatic transition and vibrational-translational exchange. The calculated probability of the migration of hydrogen by these mechanisms is found to agree well with the experimental data.

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